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Evaluation of H<sub>2sub> on the Evolution Mechanism of NO<sub><i>xi>sub> Storage and Reductionover Pt–Ba–Ce/γ-Al<sub>2sub>O<sub>3sub> Catalysts Article

Pan Wang, Jing Yi, Chuan Sun, Peng Luo, Lili Lei

Engineering 2019, Volume 5, Issue 3,   Pages 568-575 doi: 10.1016/j.eng.2019.02.005

Abstract:

In this investigation, Pt–Ba–Ce/γ-Al<sub>2sub>O<sub>3sub> catalysts were preparedThe physical and chemical properties of the Pt–Ba–Ce/γ-Al<sub>2sub>O<sub>3sub>>xsub>, CeO<sub>2sub>, and BaCO<sub>3sub>, whose peaks were observed in X-ray diffraction>catsub> at 350 °C, which was ascribed to the increase in NO<sub>2sub> yield.and conversion were increased when the time of H<sub>2sub> exposure (i.e., 30 s, 45 s, and 60 s) was

Keywords： Pt–Ba–Ce/γ-Al<sub>2sub>O<sub>3sub> catalysts     Physicochemical properties     NO<sub><i>xi>sub> storageand reduction     NO<sub><i>xi>sub> emission     H<sub>2sub> reductant    

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NO<sub><i>xi>sub> and H<sub>2sub>S formation in the reductive zone of air-staged combustion of

Jinzhi CAI, Dan LI, Denggao CHEN, Zhenshan LI

Frontiers in Energy 2021, Volume 15, Issue 1,   Pages 4-13 doi: 10.1007/s11708-020-0804-y

Abstract: Low NO combustion of blended coals is widely used in coal-fired boilers in China to control NO emission; thus, it is necessary to understand the formation mechanism of NO and H S during the combustion of blended coals. This paper focused on the investigation of reductive gases in the formation of NO and H S in the reductive zone of blended coals during combustion. Experiments with Zhundong (ZD) and Commercial (GE) coal and their blends with different mixing ratios were conducted in a drop tube furnace at 1200°C–1400°C with an excessive air ratio of 0.6–1.2. The coal conversion and formation characteristics of CO, H S, and NO in the fuel-rich zone were carefully studied under different experimental conditions for different blend ratios. Blending ZD into GE was found to increase not only the coal conversion but also the concentrations of CO and H S as NO reduction accelerated. Both the CO and H S concentrations inblended coal combustion increase with an increase in the combustion temperature and a decrease in the excessive air ratio. Based on accumulated experimental data, one interesting finding was that NO and H S from blended coal combustion were almost directly dependent on the CO concentration, and the CO concentration of the blended coal combustion depended on the single char gasification conversion.Thus, CO, NO , and H S formation characteristics from blended coal combustion can be well predicted by single char gasification kinetics.

Keywords： blended coal combustion     NO<sub><i>x i>sub>formation     H<sub>2sub>S formation     air staged combustion    

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Effects of Pd doping on N

Mingxin Dong, Jun Wang, Jinxin Zhu, Jianqiang Wang, Wulin Wang, Meiqing Shen

Frontiers of Environmental Science & Engineering 2017, Volume 11, Issue 6, doi: 10.1007/s11783-017-0976-9

Abstract: N O is a powerful greenhouse gas and plays an important role in destructing the ozone layer. This present work investigated the effects of Pd doping on N O formation over Pt/BaO/Al O catalyst. Three types of catalysts, Pt/BaO/Al O , Pt/Pd mechanical mixing catalyst (Pt/BaO/Al O +Pd/Al O ) and Pt-Pd co-impregnation catalyst (Pt-Pd/BaO/Al O ) were prepared by incipient wetness impregnation method. These catalysts were first evaluated in NSR activity tests using H /CO as reductants and then carefully characterized by BET, CO chemisorption, CO-DRIFTs and H -TPR techniques. In addition, temperature programmed reactions of NO with H /CO were conducted to obtain further information about N O formation mechanism. Compared with Pt/BaO/Al O , (Pt/BaO/Al O +Pd/Al O ) produced less N O and more NH during NO storage and reduction process, while an opposite trend was found over (Pt-Pd/BaO/Al O +Al O ). Temperature programmed reactions of NO with H /CO results showed that Pd/Al O component in (Pt/BaO/Al O +Pd/Al O ) played an important role in NO reduction to NH , and the formed NH could reduce NO to N leading to a decrease in N O formation. Most of N O formed over (Pt-Pd/BaO/Al O +Al O ) was originated from Pd/BaO/Al O component. H -TPR results indicated Pd-Ba interaction resulted in more difficult-to-reduce PdO species over Pd/BaO/Al O , which inhibits the NO dissociation and thus drives the selectivity to N O in NO reduction.

Keywords： NO<sub><i>xi>sub> storage reduction     Pt/BaO/Al<sub>2sub>O<sub>3sub>     Pd doping     N<sub>2sub>O formation    

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Simultaneous removal of NO and chlorobenzene on VO/TiO granular catalyst: Kinetic study and performance prediction

Frontiers of Environmental Science & Engineering 2021, Volume 15, Issue 4, doi: 10.1007/s11783-020-1363-5

Abstract:

• A V<sub>2sub>O<sub>5sub>/TiO<sub>2sub> granular catalyst for

Keywords： NO<sub><i>xi>sub>     Chlorobenzene     Simultaneous removal     Kinetic study     Performance prediction     V<sub>2sub>O<sub>5sub>/TiO<sub>2sub>     Graphical abstract    

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><i>In situi> growth of phosphorized ZIF-67-derived amorphous CoP/Cu<sub>2sub>O@CF electrocatalyst

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 10,   Pages 1430-1439 doi: 10.1007/s11705-023-2320-1

Abstract: Herein, we report an <i>in situi> phosphorization of zeolitic imidazole frameworks (ZIF-67) to generateThe intermediate product was phosphorized to obtain final electrocatalyst (CoP/Cu<sub>2sub>O@CF) withThe electrochemical measurement proved that CoP/Cu<sub>2sub>O@CF catalyst exhibited excellent HER activitydi>-band center of CoP downshifted after bonding with ZIF-67 and the Gibbs free energy (Δ<i>Gi><subThis work illustrates the efficient HER activity of CoP/Cu<sub>2sub>O@CF catalyst, which will act as

Keywords： CoP/Cu<sub>2sub>O@CF     electrocatalyst     phosphorization     HER     DFT    

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Preparation and characterization of lithium

Chang WANG,Yanlong ZHAI,Xi WANG,Ming ZENG

Frontiers of Chemical Science and Engineering 2014, Volume 8, Issue 4,   Pages 471-477 doi: 10.1007/s11705-014-1449-3

Abstract: Lithium -MnO ion-sieves were prepared from spinel LiMn O via treatment with nitric acid. The LiMn O was synthesized by a solid state reaction between LiOH·H O and MnO . The effects of the calcination time and temperature on the preparation of the LiMn O precursor and the lithium ion-sieve were investigated. In addition, the Li extraction ratio, the Mn dissolving ratio and the adsorption properties of the lithium ion-sieve were all measured. The lithium ion-sieve had a high exchange capacity and was selective for Li . Specifically, at pH= 13, the ion exchange capacity of Li was 30.9 mg/g in 10 mmol/L LiCl solution and the lithium extraction ratio and manganese dissolving ratio were 95% and 25%, respectively.

Keywords： lithium ion-sieve     solid state reaction     adsorption     LiMn<sub>2sub>O<sub>4sub>    

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Does environmental infrastructure investment contribute to emissions reduction? A case of China

Xiaoqian SONG, Yong GENG, Ke LI, Xi ZHANG, Fei WU, Hengyu PAN, Yiqing ZHANG

Frontiers in Energy 2020, Volume 14, Issue 1,   Pages 57-70 doi: 10.1007/s11708-019-0654-7

Abstract: Environmental infrastructure investment (EII) is an important environmental policy instrument on responding to greenhouse gas (GHG) emission and air pollution. This paper employs an improved stochastic impact by regression on population, affluence and technology (STRIPAT) model by using panel data from 30 Chinese provinces and municipalities for the period of 2003–2015 to investigate the effect of EII on CO emissions, SO emissions, and PM pollution. The results indicate that EII has a positive and significant effect on mitigating CO emission. However, the effect of EII on SO emission fluctuated although it still contributes to the reduction of PM pollution through technology innovations. Energy intensity has the largest impact on GHG emissions and air pollution, followed by GDP per capita and industrial structure. In addition, the effect of EII on environmental issues varies in different regions. Such findings suggest that policies on EII should be region-specific so that more appropriate mitigation policies can be raised by considering the local realities.

Keywords： environmental infrastructure investment (EII)     CO<sub>2sub> emission     SO<sub>2sub> emission     PM<sub>2.5sub> pollution     stochastic impact by regression on population     affluence and technology (STIRPAT)    

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grown TiN/N-TiO composite for enhanced photocatalytic H evolution activity

Frontiers in Energy 2021, Volume 15, Issue 3,   Pages 721-731 doi: 10.1007/s11708-021-0766-8

Abstract: Titanium nitride (TiN) decorated N-doped titania (N-TiO<sub>2sub>) composite (TiN/N-TiO<sub>2sub>) is fabricated via an <i>in situ i>nitridation using a hydrothermally synthesized TiO<sub>2sub>After the optimization of the reaction condition, the resultant TiN/N-TiO<sub>2sub> composite delivers>2sub> and TiN alone, respectively./N-doped TiO<sub>2sub> composite photocatalysts for high-efficiency water splitting.

Keywords： photocatalytic H<sub>2sub> evolution     TiN/N-TiO<sub>2sub> composite     plasmonic effect     <i>in-situi> nitridation    

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CeO doping boosted low-temperature NH-SCR activity of FeTiO catalyst: A microstructure analysis and reaction mechanistic study

Frontiers of Environmental Science & Engineering 2022, Volume 16, Issue 5, doi: 10.1007/s11783-022-1539-2

Abstract:

• CeO<sub>2sub> doping significantly improved low-temperature NH<sub>3sub>-SCR activity on FeTiO<sub><i>xi>sub>.

Keywords： NH<sub>3sub>-SCR     CeO<sub>2sub> doping     Low-temperature NO<sub><i>xi>sub> removal     Improved redoxproperty     <i>In situi> XAFS analysis    

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Tailoring the simultaneous abatement of methanol and NO on Sb-Ce-Zr catalysts via copper modification

Frontiers of Environmental Science & Engineering 2022, Volume 16, Issue 10, doi: 10.1007/s11684-022-1565-0

Abstract:

● Cu addition enhances CH<sub>3sub>OH oxidation and alleviates

Keywords： Copper modification     Sb-CeZr<sub>2sub>O<sub><i>xi>sub> catalyst     NO<sub><i>xi>sub>     Methanol    

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Photosynthesis and related metabolic mechanism of promoted rice (<i>Oryza sativai> L.) growth by TiO<sub>2sub> nanoparticles

Yingdan Zhang, Na Liu, Wei Wang, Jianteng Sun, Lizhong Zhu

Frontiers of Environmental Science & Engineering 2020, Volume 14, Issue 6, doi: 10.1007/s11783-020-1282-5

Abstract: Abstract • The rice growth was promoted by nano-TiO2 of 0.1–100 mg/L. • Nano-TiO2 enhanced the energystorage in photosynthesis. • Nano-TiO2 reduced energy consumption in carbohydrate metabolism and TCATitanium dioxide nanoparticle (nano-TiO2), as an excellent UV absorbent and photo-catalyst, has beenWe proposed that nano-TiO2 in soil can promote crop yield through photosynthetic and metabolic disturbanceResults showed that rice biomass was increased >30% at every applied dosage (0.1–100 mg/L) of nano-TiO2.

Keywords： Nano-TiO<sub>2sub>     Rice     Photosynthesis     Metabolomics     Energy storage    

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photocatalytic performance through the evolution of the properties due to the phase transition from NaBiO·2HO

Frontiers in Energy 2022, Volume 16, Issue 3,   Pages 471-482 doi: 10.1007/s11708-021-0778-4

Abstract: The phase transition process of a photocatalytic system from NaBiO<sub>3sub>·2H<sub>2sub>O to BiO<sub>2–sub><sub><i>xi>sub> has been investigated to understand the important factors that affectIt is found that a proper amount of BiO<sub>2–sub><sub><i>xi>sub> on the surface of NaBiO<sub>3A fully covered BiO<sub>2–sub><sub><i>xi>sub> on NaBiO<sub>3sub>·2H<sub>2sub>O results in aAn over long hydrothermal process can result in BiO<sub>2–sub><sub><i>xi>sub> with reduced oxygen

Keywords： composite construction     distribution     BiO<sub>2–sub><sub><i>xi>sub>     evolution of defects    

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Uncovering CO<sub>2sub> emission drivers under regional industrial transfer in China’s Yangtze River

Huijuan JIANG, Yong GENG, Xu TIAN, Xi ZHANG, Wei CHEN, Ziyan GAO

Frontiers in Energy 2021, Volume 15, Issue 2,   Pages 292-307 doi: 10.1007/s11708-020-0706-z

Abstract: With the relocation of heavy industries moving from downstream region to upstream and midstream regions in the Yangtze River Economic Belt (YREB), it is critical to encourage coordinated low carbon development in different regions within the YREB. This paper uncovers the evolution of CO emissions in different regions within the YREB for the period of 2000–2017. It decomposes regional CO emission changes using the temporal and cross-regional three-layer logarithmic mean Divisia index (LMDI) method. Besides, it decomposes industrial CO emission changes using the temporal two-layer LMDI method. The research results show that economic growth is the major driver for regional CO emission disparities. The mitigation drivers, such as energy intensity and energy structure, lead to a more decreased CO emission in the downstream region than in the upstream and midstream regions. In addition, it proposes several policy recommendations based upon the local realities, including improving energy efficiency, optimizing energy structure, promoting advanced technologies and equipment transfers, and coordinating the development in the upstream, midstream and downstream regions within the YREB.

Keywords： CO<sub>2sub> emission     multi-layer LMDI decomposition     industrial transfer     governance    

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Rh<sub>2sub>O<sub>3sub>/hexagonal CePO<sub>4sub> nanocatalysts for N<sub>2sub>O decomposition

Huan Liu, Zhen Ma

Frontiers of Chemical Science and Engineering 2017, Volume 11, Issue 4,   Pages 586-593 doi: 10.1007/s11705-017-1659-6

Abstract: Hexagonal CePO nanorods were prepared by a precipitation method and hexagonal CePO nanowires were prepared by hydrothermal synthesis at 150 °C. Rh(NO ) was then used as a precursor for the impregnation of Rh O onto these CePO materials. The Rh O supported on the CePO nanowires was much more active for the catalytic decomposition of N O than the Rh O supported on CePO nanorods. The stability of both catalysts as a function of time on stream was studied and the influence of the co-feed (CO , O , H O or O /H O) on the N O decomposition was also investigated. The samples were characterized by N adsorption-desorption, inductively coupled plasma optical emission spectroscopy, X-ray diffraction, transmission electron microscopy, X-ray photoelectron microscopy, hydrogen temperature-programmed reduction, oxygen temperature-programmed desorption, and CO temperature-programmed desorption in order to correlate the physicochemical and catalytic properties.

Keywords： Rh<sub>2sub>O<sub>3sub>     CePO<sub>4sub>     N<sub>2sub>O decomposition    

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Morphology selective construction of

Maher Darwish, Ali Mohammadi, Navid Assi, Samer Abuzerr, Youssef Alahmad

Frontiers of Chemical Science and Engineering 2020, Volume 14, Issue 4,   Pages 561-578 doi: 10.1007/s11705-019-1808-1

Abstract: Changing the pH of the precursor solution impacted the formation of 0D, 2D, and 3D structures; however

Keywords： <i>βi>-cyclodextrin     Bi<sub>2sub>WO<sub>6sub>     shape controlled     nanorod     sunset yellow    

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Title Author Date Type Operation

Evaluation of H<sub>2sub> on the Evolution Mechanism of NO<sub><i>xi>sub> Storage and Reductionover Pt–Ba–Ce/γ-Al<sub>2sub>O<sub>3sub> Catalysts

Pan Wang, Jing Yi, Chuan Sun, Peng Luo, Lili Lei

Journal Article

NO<sub><i>xi>sub> and H<sub>2sub>S formation in the reductive zone of air-staged combustion of

Jinzhi CAI, Dan LI, Denggao CHEN, Zhenshan LI

Journal Article

Effects of Pd doping on N

Mingxin Dong, Jun Wang, Jinxin Zhu, Jianqiang Wang, Wulin Wang, Meiqing Shen

Journal Article

Simultaneous removal of NO and chlorobenzene on VO/TiO granular catalyst: Kinetic study and performance prediction

Journal Article

><i>In situi> growth of phosphorized ZIF-67-derived amorphous CoP/Cu<sub>2sub>O@CF electrocatalyst

Journal Article

Preparation and characterization of lithium

Chang WANG,Yanlong ZHAI,Xi WANG,Ming ZENG

Journal Article

Does environmental infrastructure investment contribute to emissions reduction? A case of China

Xiaoqian SONG, Yong GENG, Ke LI, Xi ZHANG, Fei WU, Hengyu PAN, Yiqing ZHANG

Journal Article

grown TiN/N-TiO composite for enhanced photocatalytic H evolution activity

Journal Article

CeO doping boosted low-temperature NH-SCR activity of FeTiO catalyst: A microstructure analysis and reaction mechanistic study

Journal Article

Tailoring the simultaneous abatement of methanol and NO on Sb-Ce-Zr catalysts via copper modification

Journal Article

Photosynthesis and related metabolic mechanism of promoted rice (<i>Oryza sativai> L.) growth by TiO<sub>2sub> nanoparticles

Yingdan Zhang, Na Liu, Wei Wang, Jianteng Sun, Lizhong Zhu

Journal Article

photocatalytic performance through the evolution of the properties due to the phase transition from NaBiO·2HO

Journal Article

Uncovering CO<sub>2sub> emission drivers under regional industrial transfer in China’s Yangtze River

Huijuan JIANG, Yong GENG, Xu TIAN, Xi ZHANG, Wei CHEN, Ziyan GAO

Journal Article

Rh<sub>2sub>O<sub>3sub>/hexagonal CePO<sub>4sub> nanocatalysts for N<sub>2sub>O decomposition

Huan Liu, Zhen Ma

Journal Article

Morphology selective construction of

Maher Darwish, Ali Mohammadi, Navid Assi, Samer Abuzerr, Youssef Alahmad

Journal Article